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Probability of rolling a seven is 1 / 6. Probability of rolling a 2 is 1 / 36.
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The bulk of the values is around the middle numbers such as 5 through 9. 100 rolls is not efficient to determine the frequency.
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The highest frequency of values are still 5 through 9 but they seem to overall be closer.
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At 500,000 rolls you can accurately predict the probability of rolling a 7 to 3 significant digits. At 300,00 rolls you can accurately predict the probability of rolling a 2 to 3 significant digits.